There are many questions that need to be answered. What are your current diff & portal ratios? What is your tire size? Is your current top speed limited by rpms or by power? Where do you live, what kind of driving do you do?
Tearing 4 portals apart and changing gears is very expensive and a lot of work. Likewise 2 diffs. If, for example, you have 12.5-20s, changing to 365/80R20s or even bigger tires could by much easier, cheaper, and add to the offroad ability of your vehicle, and probably improve the ride. For example, changing from 12.5s to 395/85R20s is analagous to changing axle ratio from 7.5 to 6.6; 15% increase in road speed, 13% decrease in rear wheel torque.
Charlie